The Timm DCAU will probably always rank as the single best animated interpretation of a superhero franchise (although I gotta admit, Spectacular Spider-Man is right up there, or at least probably will be if it gets a third season). I quite enjoy Brave and the Bold too, just because it goes into a lot of really obscure characters. And The Batman from a couple years back is actually pretty damn fun, too, once I finally got past the art style.
Overall, I gotta say DC has had way better luck with their cartoon franchises than Marvel. Definitely more hits than misses, the crappy old Superfriends cartoon notwithstanding.
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