I don't recall seeing it as an option to play, no. And the thing with PS Now is it (stupidly) doesn't allow people while in a game on the service to go to PS Store to download add-ons. You have to do it from the dashboard. I can't count how many times I've had to be at the main PS4 screen just to download a new DLC for TESO, for example.
Also, I know this poll is about SH2, but I did start SH3 HD, and never got very far. I do hope to have a chance to play through it someday and at least beat the story once. However, I've also heard that fans of the series seem to agree that's where the series begins its gradual decline in quality.
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