You can buy Titanite shards from the first blacksmith you encounter, think they are only 500 souls or something. You can get Large Titanite Shards from a merchant near the end of Sen's Fortress too, 4000 souls a pop I believe.
I haven't played in a while since starting Skyrim, I was quite near the end of the game but I haven't got time to play both. It's weird because I'm not particularly enjoying Skyrim in gameplay terms but I feel the need to progress through the world.
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